Search results for "nonequilibrium bandstructure"

showing 2 items of 2 documents

Phonon Driven Floquet Matter.

2018

The effect of electron–phonon coupling in materials can be interpreted as a dressing of the electronic structure by the lattice vibration, leading to vibrational replicas and hybridization of electronic states. In solids, a resonantly excited coherent phonon leads to a periodic oscillation of the atomic lattice in a crystal structure bringing the material into a nonequilibrium electronic configuration. Periodically oscillating quantum systems can be understood in terms of Floquet theory, which has a long tradition in the study of semiclassical light-matter interaction. Here, we show that the concepts of Floquet analysis can be applied to coherent lattice vibrations. This coupling leads to p…

Floquet theoryFloquet theoryPhononphotoelectron spectroscopynonequilibrium bandstructureFOS: Physical sciencesSemiclassical physicsBioengineeringAngle-resolved photoemission spectroscopy02 engineering and technologyElectronic structureelectron?phonon coupling01 natural sciencesSettore FIS/03 - Fisica Della MateriaFirst-principles calculations0103 physical sciencesGeneral Materials Science010306 general physicsElectronic band structurePhysicsCondensed Matter - Materials Sciencepumpprobe spectroscopyCondensed matter physicsMechanical EngineeringMaterials Science (cond-mat.mtrl-sci)General Chemistry021001 nanoscience & nanotechnologyCondensed Matter PhysicsExcited stateElectron configuration0210 nano-technologyNano letters
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Monitoring Electron-Photon Dressing in WSe 2

2016

Optical pumping of solids creates a non-equilibrium electronic structure where electrons and photons combine to form quasiparticles of dressed electronic states. The resulting shift of electronic levels is known as the optical Stark effect, visible as a red shift in the optical spectrum. Here we show that in a pump-probe setup we can uniquely define a non-equilibrium quasiparticle bandstructure that can be directly measurable with photoelectron spectroscopy. The dynamical photon-dressing (and undressing) of the many-body electronic states can be monitored by pump-probe time and angular resolved photoelectron spectroscopy (tr-ARPES) as the photon-dressed bandstructure evolves in time dependi…

Floquet theoryFloquet theoryPhotonphotoelectron spectroscopynonequilibrium bandstructurePhysics::OpticsBioengineering02 engineering and technologyElectronElectronic structure01 natural sciencesSettore FIS/03 - Fisica Della MateriaOptical pumpingsymbols.namesakeFirst-principles calculations0103 physical sciencesGeneral Materials Science010306 general physicsChemistryMechanical Engineeringpump-probe spectroscopyGeneral Chemistry021001 nanoscience & nanotechnologyCondensed Matter PhysicsStark effectQuasiparticlesymbolsCondensed Matter::Strongly Correlated ElectronsAtomic physics0210 nano-technologyVisible spectrumNano Letters
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